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Electronic structure and reactivity of low-spin Fe(III)-hydroperoxo complexes: comparison to activated bleomycin.
Lehnert N, Neese F, Ho RY, Que L Jr, Solomon EI. Lehnert N, et al. Among authors: neese f. J Am Chem Soc. 2002 Sep 11;124(36):10810-22. doi: 10.1021/ja012621d. J Am Chem Soc. 2002. PMID: 12207537
In contrast, ABLM has a somewhat different electronic structure where no pi donor bond between the hydroperoxo ligand and iron(III) is present [Neese, F.; Zaleski, J. M.; Loeb-Zaleski, K.; Solomon, E. I. J. Am. Chem. Soc. 2000, 122, 11703]. ...
In contrast, ABLM has a somewhat different electronic structure where no pi donor bond between the hydroperoxo ligand and iron(III) is prese …
Characterization of a genuine iron(V)-nitrido species by nuclear resonant vibrational spectroscopy coupled to density functional calculations.
Petrenko T, DeBeer George S, Aliaga-Alcalde N, Bill E, Mienert B, Xiao Y, Guo Y, Sturhahn W, Cramer SP, Wieghardt K, Neese F. Petrenko T, et al. Among authors: neese f. J Am Chem Soc. 2007 Sep 12;129(36):11053-60. doi: 10.1021/ja070792y. Epub 2007 Aug 21. J Am Chem Soc. 2007. PMID: 17711275
.; DeBeer George, S.; Bill, E.; Wieghardt, K.; Neese, F. Angew. Chem., Int. Ed. 2005, 44, 2908-2912). The results of this study indicated that the [Fe(V)-nitrido-cyclam-acetato]+ complex is an unusual d3 system with a nearly orbitally degenerate S=1/2 ground state. …
.; DeBeer George, S.; Bill, E.; Wieghardt, K.; Neese, F. Angew. Chem., Int. Ed. 2005, 44, 2908-2912). The results of this stud …
546 results