Monomeric bovine beta-lactoglobulin adopts a beta-barrel fold at pH 2

FEBS Lett. 1998 Oct 2;436(2):149-54. doi: 10.1016/s0014-5793(98)00936-3.

Abstract

We have determined a crude structure of the apo form of bovine beta-lactoglobulin, a protein of 162 amino acid residues with a molecular mass of 18 kDa, at a low pH on the basis of data collected using only homonuclear 1H NMR spectroscopy. An ensemble of protein conformations was calculated with the distance-geometry algorithm for NMR applications (DYANA). The monomeric protein at low pH adopts a beta-barrel fold, well-superimposable on the structure determined by X-ray crystallography for the dimer at physiological pH. NMR evidence suggests the presence of disordered loop regions and terminal segments. Structural differences between the monomer at pH 2 and the dimer at pH 7, obtained by X-ray crystallography, are discussed, paying particular attention to surface electrostatic properties, in view of the high charge state of the protein at low pH.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Algorithms
  • Amino Acid Sequence
  • Animals
  • Apoproteins / chemistry
  • Cattle
  • Crystallography, X-Ray
  • Hydrogen-Ion Concentration
  • Lactoglobulins / chemistry*
  • Models, Molecular
  • Molecular Sequence Data
  • Nuclear Magnetic Resonance, Biomolecular
  • Protein Conformation
  • Protein Folding*
  • Protein Structure, Secondary*
  • Static Electricity

Substances

  • Apoproteins
  • Lactoglobulins