The bilirubin-binding motif of bilitranslocase and its relation to conserved motifs in ancient biliproteins

Biochem Biophys Res Commun. 1998 Jun 29;247(3):687-92. doi: 10.1006/bbrc.1998.8868.

Abstract

In the primary structure of bilitranslocase, currently under study in our laboratory, an aminoacid motif was identified and found to be conserved in a number of alpha-phycocyanines, ancient biliproteins present in cyanobacteria. To test the possibility that such a motif could be at least part of the binding site for bilirubin, epitope-specific antibodies were raised. The target corresponds to the sequence 65-75 of bilitranslocase and covers the central portion of the motif identified. The antibodies were shown: 1) to inhibit the electrogenic BSP transport by plasmamembrane vesicles; 2) to react with purified bilitranslocase; and 3) to identify only one protein band with electrophoretic mobility identical to bilitranslocase in Western blots of solubilised plasmamembrane vesicles. The presence of either bilirubin or nicotinate during pre-incubation with the antibodies decreases concentration-wise the inhibition kinetics. From these experiments a dissociation constant of 2.2 +/- 0.3 and 11.3 +/- 1.3 nM for bilirubin-bilitranslocase and nicotinate-bilitranslocase complexes were calculated.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Animals
  • Antibodies / pharmacology
  • Bilirubin / metabolism*
  • Binding Sites / genetics
  • Biological Transport
  • Ceruloplasmin
  • Conserved Sequence / genetics
  • Epitopes / chemistry
  • Kinetics
  • Liver / physiology
  • Membrane Proteins / chemistry*
  • Membrane Proteins / immunology
  • Molecular Sequence Data
  • Molecular Structure
  • Niacin / metabolism
  • Peptide Fragments / immunology
  • Phycocyanin / analogs & derivatives
  • Phycocyanin / chemistry
  • Protein Binding / physiology
  • Rats
  • Sequence Homology, Amino Acid
  • Sulfobromophthalein / metabolism

Substances

  • Antibodies
  • Epitopes
  • Membrane Proteins
  • Peptide Fragments
  • Sulfobromophthalein
  • Phycocyanin
  • Niacin
  • Ceruloplasmin
  • bilitranslocase
  • Bilirubin

Associated data

  • GENBANK/Y12178