Antioxidant activity of lazaroid (U-75412E) and its protective effects against crystalline silica-induced cytotoxicity

Free Radic Biol Med. 1998 Mar 1;24(4):529-36. doi: 10.1016/s0891-5849(97)00285-2.

Abstract

Lazaroids (21-amino steroids) are believed to be powerful scavengers of reactive oxygen species (ROS) and inhibitors of lipid peroxidation. Crystalline silica, a potent cytotoxic agent, causes pulmonary fibrosis in experimental animals and humans. ROS have been previously shown to be involved in crystalline silica-induced pulmonary injury and inflammation. In the present study, the reaction rate of lazaroid (U-75412E) with hydroxyl radical (.OH) generated by Fenton reaction (Fe(II) + H2O2 --> Fe(III) + OH- + .OH) was investigated using ESR spin-trapping competition reactions. The reaction rate constant was found to be 1.0 x 10(10) M(-1)s(-1), which was comparable with those of other efficient .OH radical scavengers. As indicators of crystalline silica-induced cytotoxicity and its protection by this antioxidant lazaroid (U-75412E) we measured lactate dehydrogenase, N-acetyl-beta-glucosaminidase, superoxide dismutase, glutathione peroxidase, and hydrogen peroxide released from rat alveolar macrophages. Lipid peroxidation, a prominent manifestation of .OH radical-induced cell injury, was also measured to evaluate the protective value of lazaroid. Alveolar macrophages treated with lazaroid (U-75412E) before crystalline silica exposure were protected against cell injury and lipid peroxidation as demonstrated by those indicators. Lazaroid (U-75412E) scavenges .OH radicals generated by crystalline silica-mediated reaction from H2O2 and inhibits lipid peroxidation in macrophages induced by these particles.

MeSH terms

  • Animals
  • Antioxidants / pharmacology*
  • Crystallization
  • Cyclic N-Oxides / chemistry
  • Electron Spin Resonance Spectroscopy
  • Free Radical Scavengers / pharmacology
  • Hydrogen Peroxide / metabolism
  • Hydroxyl Radical / metabolism
  • Kinetics
  • Lipid Peroxidation / drug effects
  • Macrophages, Alveolar / drug effects
  • Macrophages, Alveolar / metabolism
  • Male
  • Rats
  • Rats, Sprague-Dawley
  • Silicon Dioxide / chemistry
  • Silicon Dioxide / toxicity*
  • Spin Labels
  • Steroids / pharmacology*
  • Thiobarbituric Acid Reactive Substances / metabolism

Substances

  • Antioxidants
  • Cyclic N-Oxides
  • Free Radical Scavengers
  • Spin Labels
  • Steroids
  • Thiobarbituric Acid Reactive Substances
  • U 75412E
  • Hydroxyl Radical
  • 5,5-dimethyl-1-pyrroline-1-oxide
  • Silicon Dioxide
  • Hydrogen Peroxide