Identification of a chloroquine importer in Plasmodium falciparum. Differences in import kinetics are genetically linked with the chloroquine-resistant phenotype

J Biol Chem. 1997 Jan 31;272(5):2652-8. doi: 10.1074/jbc.272.5.2652.

Abstract

We demonstrate that uptake of the antimalarial drug chloroquine is temperature-dependent, saturable, and inhibitable in Plasmodium falciparum. These features are indicative of carrier-mediated transport and suggest that a P. falciparum-encoded protein facilitates chloroquine import. Although both chloroquine-resistant and susceptible parasite isolates exhibit facilitated chloroquine uptake, the kinetics differ. Chloroquine-resistant parasite isolates consistently have an import mechanism with a lower transport activity and a reduced affinity for chloroquine. These differences in uptake kinetics are linked with chloroquine resistance in a genetic cross. These data suggest that changes in chloroquine import kinetics constitute a minimal and necessary event in the generation of the resistant phenotype. Competitive inhibition of chloroquine uptake by amiloride derivatives further suggests that chloroquine import is mediated by a plasmodial Na+/H+ exchanger.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amiloride / analogs & derivatives
  • Amiloride / pharmacology
  • Animals
  • Binding, Competitive
  • Biological Transport / drug effects
  • Chloroquine / metabolism*
  • Chloroquine / toxicity*
  • Crosses, Genetic
  • Drug Resistance / genetics*
  • Erythrocytes / metabolism
  • Humans
  • Kinetics
  • Phenotype
  • Plasmodium falciparum / drug effects
  • Plasmodium falciparum / genetics
  • Plasmodium falciparum / metabolism*
  • Sodium-Hydrogen Exchangers / metabolism*
  • Temperature

Substances

  • Sodium-Hydrogen Exchangers
  • Amiloride
  • Chloroquine
  • ethylisopropylamiloride