Solid-phase extraction and gas chromatographic-mass spectrometric determination after hydrolysis of 2-aminofluorene haemoglobin adducts in blood of rats

J Chromatogr. 1993 Sep 22;619(2):215-21. doi: 10.1016/0378-4347(93)80110-p.

Abstract

2-Nitrofluorene is an environmental pollutant that binds covalently to haemoglobin after nitroreduction and successive N-hydroxylation. these haemoglobin adducts can be cleaved in vitro by mild base-catalysed hydrolysis. For the enrichment of arylamines from the aqueous hydrolysate, an extraction procedure with an organic solvent is widely used. Because of the formation of a thick emulsion layer between the aqueous and organic solvent layers, the extraction is laborious and inefficient. The use of Amberlite XAD2 provides a simple extraction procedure yielding a recovery of ca. 70%. Calibration curves in haemoglobin solution were prepared with a correlation coefficient of 0.998 (n = 12). The inter-day coefficient of variation amounted to 14%.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Cysteine / analysis
  • Female
  • Fluorenes / blood*
  • Gas Chromatography-Mass Spectrometry
  • Hemoglobins / analysis*
  • Hydrolysis
  • Indicators and Reagents
  • Male
  • Rats
  • Rats, Wistar
  • Solvents

Substances

  • Fluorenes
  • Hemoglobins
  • Indicators and Reagents
  • Solvents
  • 2-aminofluorene
  • Cysteine