Purification and characterization of a ubenimex (Bestatin)-sensitive aminopeptidase B-like enzyme from K562 human chronic myeloid leukemia cells

FEBS Lett. 1994 Mar 28;342(1):53-6. doi: 10.1016/0014-5793(94)80583-0.

Abstract

A ubenimex-sensitive aminopeptidase B-like enzyme was purified from the non-membrane-bound fraction of K562 cells by a series of chromatographic procedures and slab-gel electrophoresis. The apparent molecular mass of the enzyme was estimated to be 73 kDa by SDS-PAGE. The aminopeptidase activity was activated by chloride ions and inhibited by Zn2+, Cu2+, Cd2+, and p-chloromercuribenzoic acid. Ubenimex was a potent inhibitor of this aminopeptidase in the nanomolar range. The sequence of the N-terminus of the protein was not determined. Partial amino acid sequencing revealed that the N-terminus of this aminopeptidase B-like enzyme was blocked by acylation. The partial sequences of the two fragments produced by CNBr cleavage and an acylamino acid-releasing reaction showed this enzyme to be a new aminopeptidase.

MeSH terms

  • Amino Acid Sequence
  • Aminopeptidases / antagonists & inhibitors
  • Aminopeptidases / chemistry
  • Aminopeptidases / isolation & purification*
  • Aminopeptidases / metabolism
  • Cations, Divalent / pharmacology
  • Chlorides / pharmacology
  • Humans
  • Hydrogen-Ion Concentration
  • Leucine / analogs & derivatives*
  • Leucine / pharmacology
  • Leukemia, Myelogenous, Chronic, BCR-ABL Positive / enzymology*
  • Molecular Sequence Data
  • Molecular Weight
  • Substrate Specificity
  • Tumor Cells, Cultured

Substances

  • Cations, Divalent
  • Chlorides
  • Aminopeptidases
  • aminopeptidase B
  • Leucine
  • ubenimex