Analysis by limited proteolysis of domain organization and GSH-site arrangement of bacterial glutathione transferase B1-1

Int J Biochem Cell Biol. 1995 Oct;27(10):1033-41. doi: 10.1016/1357-2725(95)00081-y.

Abstract

Limited proteolysis method has been used to study the structure-function relationship of bacterial glutathione transferase (GSTB1-1). In absence of three-dimensional structural data of prokaryote GST, the results represent the first information concerning the G-site and domains organization of GSTB1-1. The tryptic cleavages occur mainly at the peptide bonds Lys35-Lys36 and Phe43-Leu44, generating two major molecular species of 20-kDa, 3-kDa and traces of 10-kDa. 1-chloro-2,4-dinitrobenzene favoured the proteolysis of the 20-kDa fragment markedly enhancing the production of the 10-kDa peptide by cleaving the chemical bonds Lys87-Ala88 and Arg91-Tyr92. The tryptic cleavage sites of GSTB1-1 was found to be located close to those previously found for the mammalian GSTP1-1 isozyme. It was concluded that despite their low sequence homology (18%), GSTB1-1 and GSTP1-1 displayed similar structural features in their G-site regions and probably a common organization in structural domains.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Binding Sites
  • Biological Evolution
  • Chymotrypsin
  • Circular Dichroism
  • Dinitrochlorobenzene / metabolism
  • Dinitrochlorobenzene / pharmacology
  • Electrophoresis, Polyacrylamide Gel
  • Glutathione / analogs & derivatives
  • Glutathione / pharmacology
  • Glutathione Transferase / chemistry*
  • Glutathione Transferase / metabolism
  • Molecular Sequence Data
  • Peptide Fragments / chemistry
  • Peptide Fragments / metabolism
  • Protein Structure, Secondary
  • Proteus mirabilis / enzymology*
  • Sequence Homology, Amino Acid
  • Structure-Activity Relationship
  • Trypsin

Substances

  • Dinitrochlorobenzene
  • Peptide Fragments
  • Glutathione Transferase
  • Chymotrypsin
  • Trypsin
  • Glutathione
  • S-methyl glutathione