Improved biotinylation of glucose-6-phosphate dehydrogenase using active-site-blocking agents

Anal Biochem. 1985 Aug 15;149(1):225-8. doi: 10.1016/0003-2697(85)90499-3.

Abstract

Characteristics of the biotinylation of glucose-6-phosphate dehydrogenase are presented. The enzyme is inactivated in the presence of N-hydroxysuccinimido biotin but can be protected by an appropriate concentration of NADPH used as an active-site blocker. A Ki of 1.6 +/- 1.0 microM calculated for NADPH for this protection shows it to be an active-site phenomena. Enzyme inactivation is irreversible with consistent kinetic results requiring the presence of 10 mM EDTA. An improved methodology was developed for biotinylation allowing 100% protection of the enzyme with loading factors up to 30.8 mol of biotin per enzyme.

MeSH terms

  • Binding Sites / drug effects
  • Biotin* / analogs & derivatives
  • Chemical Phenomena
  • Chemistry
  • Glucosephosphate Dehydrogenase*
  • Kinetics
  • NADP
  • Succinimides

Substances

  • Succinimides
  • biotinyl N-hydroxysuccinimide ester
  • NADP
  • Biotin
  • Glucosephosphate Dehydrogenase