Child exposure to N-(1,3-dimethylbutyl)-N'-phenyl-p-phenylenediamine (6PPD) and its derived quinone (6PPDQ) in e-waste areas: Urinary concentrations, sources, and health effect assessment

J Environ Sci (China). 2025 Jul:153:217-228. doi: 10.1016/j.jes.2024.07.011. Epub 2024 Jul 27.

Abstract

N-(1,3-dimethylbutyl)-N'-phenyl-p-phenylenediamine quinone (6PPDQ) and its parent 6PPD are ubiquitous in the environment and may induce multi-endpoint toxicity. Electronic waste (e-waste) dismantling is an under-recognized source of 6PPD and 6PPDQ emissions, and there is a lack of epidemiological investigations into their presence and health effects in local populations. This study aimed to determine the urinary concentrations of 6PPD and 6PPDQ in children aged 2-7 years from e-waste dismantling areas and evaluate their potential risk to physical growth. We found that children from the e-waste area had significantly elevated urinary concentrations of 6PPD and 6PPDQ (median: 0.073 and 2.34 ng/mL) compared to those in the reference area (0.020 and 0.24 ng/mL, respectively). The estimated urinary excretions of 6PPDQ in the e-waste exposure group were considerably higher than that in the reference group (p < 0.001). Furthermore, a borderline significant association of co-exposure to high levels of 6PPD and 6PPDQ with lower BMI z-score (OR = 1.99, 95% Cl: 1.04, 3.82) was observed in the crude model and the model adjusted for age and gender. In conclusion, our study first reported the urinary 6PPD and 6PPDQ concentrations in children from e-waste dismantling areas. The result indicated that e-waste recycling activities contribute to significantly elevated body burdens of 6PPD and 6PPDQ in children, which may be a potential risk factor for physical growth. Further epidemiological and toxicological studies are needed to investigate the exposure and health risks, especially in vulnerable populations.

Keywords: 6PPDQ; Biomonitoring; Childhood; E-waste; Physical growth.

MeSH terms

  • Child
  • Child, Preschool
  • Electronic Waste*
  • Environmental Exposure / statistics & numerical data
  • Environmental Monitoring
  • Environmental Pollutants / urine
  • Female
  • Humans
  • Male
  • Phenylenediamines* / urine
  • Quinones

Substances

  • Phenylenediamines
  • Environmental Pollutants
  • Quinones