Table-top source for x-ray absorption spectroscopy with photon energies up to 350 eV

Rev Sci Instrum. 2024 Oct 1;95(10):103001. doi: 10.1063/5.0219921.

Abstract

We present a table-top setup for x-ray absorption spectroscopy (XAS) based on high harmonic generation (HHG) in noble gases. Using sub-millijoule pump pulses at a central wavelength of 1550 nm, broadband HHG in the range of 70-350 eV was demonstrated. The HHG coherence lengths of several millimeters were achieved by reaching the nonadiabatic regime of harmonic generation. Near edge x-ray absorption fine structure spectroscopy experiments on the boron K edge of a boron foil and a hexagonal boron nitride (hBN) 2D material demonstrate the capabilities of the setup. Femtosecond pulse duration makes pump-probe XAS experiments with corresponding time resolution possible.