The β-d- manno-heptoses are immune agonists across kingdoms

Science. 2024 Aug 9;385(6709):678-684. doi: 10.1126/science.adk7314. Epub 2024 Aug 8.

Abstract

Bacterial small molecule metabolites such as adenosine-diphosphate-d-glycero-β-d-manno-heptose (ADP-heptose) and their derivatives act as effective innate immune agonists in mammals. We show that functional nucleotide-diphosphate-heptose biosynthetic enzymes (HBEs) are distributed widely in bacteria, archaea, eukaryotes, and viruses. We identified a conserved STTR5 motif as a hallmark of heptose nucleotidyltransferases that can synthesize not only ADP-heptose but also cytidine-diphosphate (CDP)- and uridine-diphosphate (UDP)-heptose. Both CDP- and UDP-heptoses are agonists that trigger stronger alpha-protein kinase 1 (ALPK1)-dependent immune responses than ADP-heptose in human and mouse cells and mice. We also produced ADP-heptose in archaea and verified its innate immune agonist functions. Hence, the β-d-manno-heptoses are cross-kingdom, small-molecule, pathogen-associated molecular patterns that activate the ALPK1-dependent innate immune signaling cascade.

MeSH terms

  • Amino Acid Motifs
  • Animals
  • Archaea / enzymology
  • Bacteria / enzymology
  • Bacteria / metabolism
  • Heptoses* / biosynthesis
  • Heptoses* / immunology
  • Humans
  • Immunity, Innate
  • Mice
  • Nucleotidyltransferases* / chemistry
  • Nucleotidyltransferases* / classification
  • Nucleotidyltransferases* / genetics
  • Pathogen-Associated Molecular Pattern Molecules* / immunology
  • Pathogen-Associated Molecular Pattern Molecules* / metabolism
  • Protein Kinases / metabolism
  • Viruses / enzymology

Substances

  • Heptoses
  • Nucleotidyltransferases
  • ADP-heptose
  • Pathogen-Associated Molecular Pattern Molecules
  • Protein Kinases
  • ALPK1 protein, mouse