Simultaneous Biofilm Disruption, Bacterial Killing, and Inflammation Elimination for Wound Treatment Using Silver Embellished Polydopamine Nanoplatform

Small. 2024 Sep;20(36):e2400927. doi: 10.1002/smll.202400927. Epub 2024 May 10.

Abstract

Due to the presence of spatial barriers, persistent bacteria, and excessive inflammation in bacteria biofilm-infected wounds, current nanoplatforms cannot effectively address these issues simultaneously during the therapeutic process. Herein, a novel biomimetic photothermal nanoplatform integrating silver and polydopamine nanoparticles (Ag/PDAs) that can damage biofilms, kill bacterial persisters, and reduce inflammation for wound treatment is presented. These findings reveal that Ag/PDAs exhibit a broad-spectrum antimicrobial activity through direct damage to the bacterial membrane structure. Additionally, Ag/PDAs demonstrate a potent photothermal conversion efficiency. When combined with near-infrared (NIR) irradiation, Ag/PDAs effectively disrupt the spatial structure of biofilms and synergistically eradicate the resident bacteria. Furthermore, Ag/PDAs show remarkable anti-inflammatory properties in counteracting bacterium-induced macrophage polarization. The in vivo results confirm that the topical application of Ag/PDAs significantly suppress Staphylococcus aureus biofilm-infected wounds in murine models, concurrently facilitating wound healing. This research provides a promising avenue for the eradication of bacterial biofilms and the treatment of biofilm-infected wounds.

Keywords: bacterial biofilm; dopamine; infected wound; inflammation; photothermal.

MeSH terms

  • Animals
  • Anti-Bacterial Agents / chemistry
  • Anti-Bacterial Agents / pharmacology
  • Biofilms* / drug effects
  • Indoles* / chemistry
  • Indoles* / pharmacology
  • Inflammation* / drug therapy
  • Inflammation* / pathology
  • Mice
  • Nanoparticles / chemistry
  • Polymers* / chemistry
  • Polymers* / pharmacology
  • Silver* / chemistry
  • Silver* / pharmacology
  • Staphylococcus aureus* / drug effects
  • Wound Healing / drug effects

Substances

  • polydopamine
  • Indoles
  • Polymers
  • Silver
  • Anti-Bacterial Agents