Optimization of sample clean-up for the determination of small amounts of MOSH and MOAH in edible oils - method DGF C-VI 22 (20)

Food Addit Contam Part A Chem Anal Control Expo Risk Assess. 2023 Nov;40(11):1423-1439. doi: 10.1080/19440049.2023.2258991. Epub 2023 Nov 6.

Abstract

Methods for determining MOSH and MOAH in edible oils showed major problems with interlaboratory comparability of analytical results, especially in the lower concentration range below 10 mg/kg. However, a method with improved sensitivity and reproducibility is urgently needed to obtain a valid data basis for minimization efforts. To cope this problem a new method was created in 2020. The method was established as the standard method DGF C-VI 22 (20) of the German Society for Fat Science e.V. (DGF). For the development of this method different sample epoxidation approaches have been performed, evaluated and improved. Additionally, a saponification, a decision tree for sample preparation, an upstream clean-up column and a system suitability test were introduced. The focus was on reliability and interlaboratory comparability over all edible oil matrices up to a LOQ of 1 mg/kg. The optimized method was validated in terms of trueness and precision in a collaborative trail with 11 laboratories. The achieved recovery rates of 89-105% MOSH and 70-105% MOAH met the JRC requirements. Method and validation results were obtained with HorRat values between 1.3 and 1.8 for MOSH and MOAH.

Keywords: LC-GC-FID; MOAH; MOSH; edible oil; epoxidation; method validation; mineral oil; standard method.

MeSH terms

  • Chromatography, Gas / methods
  • Food Contamination / analysis
  • Hydrocarbons, Aromatic* / analysis
  • Mineral Oil / analysis
  • Oils
  • Reproducibility of Results

Substances

  • Hydrocarbons, Aromatic
  • Mineral Oil
  • Oils