Decarbonylation of benzaldehydes by dual photoorgano-cobalt catalysis

Chem Commun (Camb). 2023 Jul 6;59(55):8592-8595. doi: 10.1039/d3cc02170j.

Abstract

We report a mild alternative to thermally-driven noble-metal catalyzed decarbonylation protocols for the defunctionalization of benzaldehydes in short reaction times. Our cooperative photocatalytic system involves thioxanthone as an inexpensive HAT-agent and a cobalt complex required for selective C(sp2)-C(sp2) bond cleavage. The generated acyl and phenyl intermediates are postulated to be stabilized as cobalt complexes.

MeSH terms

  • Benzaldehydes* / chemistry
  • Catalysis
  • Cobalt* / chemistry

Substances

  • Cobalt
  • Benzaldehydes