Ainslides A-F, Six Sesquiterpenoids Isolated from Ainsliaea pertyoides and Their NLRP3-Inflammasome Inhibitory Activity

Chem Biodivers. 2022 May;19(5):e202200135. doi: 10.1002/cbdv.202200135. Epub 2022 Apr 5.

Abstract

Six new sesquiterpenoids, named as ainslides A-F (1-6), including one carotene-type sesquiterpene (1), one eudesmane (2), four guaianolides (3-6), together with eight known sesquiterpenoids (7-14), were purified from the whole plants of Ainsliaea pertyoides. The structures of these sesquiterpenoids were characterized based on spectroscopic methods including 1D and 2D NMR, HR-ESI-MS, UV, and IR spectra, together with ECD calculations and X-ray diffraction experiments. The anti-inflammatory activity of all the isolated compounds was screened and compounds 3 and 7-13 exhibited NLRP3-inflammasome inhibitory activity with IC50 values of 1.80-4.33 μM.

Keywords: Ainsliaea pertyoides; NLRP3 inflammasome; anti-inflammatory activity; sesquiterpenoids.

MeSH terms

  • Asteraceae* / chemistry
  • Inflammasomes
  • Molecular Structure
  • NLR Family, Pyrin Domain-Containing 3 Protein
  • Sesquiterpenes* / chemistry
  • Sesquiterpenes* / pharmacology

Substances

  • Inflammasomes
  • NLR Family, Pyrin Domain-Containing 3 Protein
  • Sesquiterpenes