Mapping the Influence of the Gut Microbiota on Small Molecules across the Microbiome Gut Brain Axis

J Am Soc Mass Spectrom. 2022 Apr 6;33(4):649-659. doi: 10.1021/jasms.1c00298. Epub 2022 Mar 9.

Abstract

Microbes exert influence across the microbiome-gut-brain axis through neurotransmitter production, induction of host immunomodulators, or the release or induction of other microbial or host molecules. Here, we used mass spectrometry imaging (MSI), a label-free imaging tool, to map molecular changes in the gut and brain in germ-free, antibiotic-treated and control mice. We determined spatial distribution and relative quantification of neurotransmitters and their precursors in response to the microbiome. Using untargeted MSI, we detected a significant change in the levels of four identified small molecules in the brains of germ-free animals compared to controls. However, antibiotic treatment induced no significant changes in these same metabolites in the brain after 1 week of treatment. This work exemplifies the utility of MSI as a tool for the study of known and discovery of novel, mediators of microbiome-gut-brain axis communication.

Keywords: brain; mass spectrometry imaging; metabolites; microbiome; neurotransmitters.

MeSH terms

  • Animals
  • Brain / metabolism
  • Brain-Gut Axis
  • Gastrointestinal Microbiome* / physiology
  • Mass Spectrometry / methods
  • Mice
  • Microbiota*