Tailoring an HSO4- anion hybrid receptor based on a phenazine derivative

Photochem Photobiol Sci. 2020 Oct 1;19(10):1373-1381. doi: 10.1039/d0pp00159g. Epub 2020 Aug 27.

Abstract

A catechol-functionalized phenazine imidazole (PD) was tailored with 2,3-diaminophenazine and 3,4-dihydroxy benzaldehyde, and it served as a hybrid acceptor for capturing HSO4- anions. The selectivity and sensitivity of the PD receptor for anion sensing were studied. It was found that the PD receptor could not only display a preferable sensitivity to HSO4- ions with a "turn-off" fluorescence response, but also have a strong anti-interference ability toward other common anions, especially basic anions such as CH3COO-, HPO42-, and H2PO4-. The anion recognition mechanism of PD towards HSO4- is based on multiple hydrogen bond interactions. Finally, the strips for anion detection were prepared, which were verified to be a convenient and high-efficiency test kit for detecting HSO4- ions with the naked eye.

MeSH terms

  • Anions / chemistry
  • Fluorescence
  • Molecular Structure
  • Particle Size
  • Phenazines / chemical synthesis
  • Phenazines / chemistry*
  • Sulfites / chemical synthesis
  • Sulfites / chemistry*
  • Surface Properties

Substances

  • Anions
  • Phenazines
  • Sulfites
  • hydrogen sulfite