Quantitative NMR-Based Metabolomics on Tissue Biomarkers and Its Translation into In Vivo Magnetic Resonance Spectroscopy

Methods Mol Biol. 2019:1978:369-387. doi: 10.1007/978-1-4939-9236-2_23.

Abstract

Nuclear magnetic resonance (NMR) spectroscopy is an established analytical platform for analyzing metabolic profiles of cells, tissues, and body fluids. There are several advantages in introducing an NMR-based study design into metabolomics studies, including a fast and comprehensive detection, characterization, and quantification of dozens of endogenous metabolites in a single NMR spectrum. Quantitative proton 1H-NMR is the most useful NMR-based platform for metabolomics. The frozen tissues can be analyzed noninvasively using a high-resolution magic angle spinning (HR-MAS) 1H-NMR spectroscopy; or several extraction techniques can be applied to detect additional metabolites using a conventional liquid-based NMR technique. In this chapter, we report on tissue collection, handling, extraction methods, and 1H-NMR acquisition protocols developed in the past decades for a precise and quantitative NMR-metabolomics approach. The NMR acquisition protocols (both HR-MAS and conventional 1H-NMR spectroscopy) and spectral analysis steps are also presented. Since NMR can be applied "in vivo" using horizontal bore MRI scanners, several in vivo sequences for localized 1H-MRS (magnetic resonance spectroscopy) are presented which can be directly applied for noninvasive detection of brain metabolites.

Keywords: Chemical shift; Endogenous metabolites; High-resolution magic angle spinning (HR-MAS); Magnetic resonance spectroscopy (MRS); Metabolite quantification; Nuclear magnetic resonance (NMR); Tissue extraction.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Biomarkers / chemistry
  • Biomarkers / metabolism*
  • Body Fluids / metabolism
  • Brain / metabolism
  • Humans
  • Magnetic Resonance Imaging / methods*
  • Metabolome / genetics
  • Metabolomics / methods*
  • Proton Magnetic Resonance Spectroscopy / methods*

Substances

  • Biomarkers