MS-based targeted metabolomics of eicosanoids and other oxylipins: Analytical and inter-individual variabilities

Free Radic Biol Med. 2019 Nov 20:144:72-89. doi: 10.1016/j.freeradbiomed.2019.05.012. Epub 2019 May 11.

Abstract

Oxylipins, including the well-known eicosanoids, are potent lipid mediators involved in numerous physiological and pathological processes. Therefore, their quantitative profiling has gained a lot of attention during the last years notably in the active field of health biomarker discovery. Oxylipins include hundreds of structurally and stereochemically distinct lipid species which today are most commonly analyzed by (ultra) high performance liquid chromatography-mass spectrometry based ((U)HPLC-MS) methods. To maximize the utility of oxylipin profiling in clinical research, it is crucial to understand and assess the factors contributing to the analytical and biological variability of oxylipin profiles in humans. In this review, these factors and their impacts are summarized and discussed, providing a framework for recommendations expected to enhance the interlaboratory comparability and biological interpretation of oxylipin profiling in clinical research.

Publication types

  • Research Support, Non-U.S. Gov't
  • Review

MeSH terms

  • Arachidonic Acid / chemistry
  • Arachidonic Acid / metabolism
  • Cardiovascular Diseases / diagnosis
  • Cardiovascular Diseases / metabolism*
  • Cardiovascular Diseases / physiopathology
  • Chromatography, High Pressure Liquid / standards*
  • Eicosanoids / analysis*
  • Eicosanoids / chemistry
  • Eicosanoids / metabolism
  • Fatty Acids, Unsaturated / chemistry
  • Fatty Acids, Unsaturated / metabolism
  • Humans
  • Inflammation
  • Metabolomics / instrumentation
  • Metabolomics / methods
  • Metabolomics / organization & administration
  • Neurodegenerative Diseases / diagnosis
  • Neurodegenerative Diseases / metabolism*
  • Neurodegenerative Diseases / physiopathology
  • Observer Variation
  • Oxylipins / analysis*
  • Oxylipins / chemistry
  • Oxylipins / metabolism
  • Reproducibility of Results
  • Tandem Mass Spectrometry / standards*
  • Vasoconstriction / physiology
  • Vasodilation / physiology

Substances

  • Eicosanoids
  • Fatty Acids, Unsaturated
  • Oxylipins
  • Arachidonic Acid