Chiral Incommensurate Helical Phase in a Smectic of Achiral Bent-Core Mesogens

Phys Rev Lett. 2019 Mar 15;122(10):107801. doi: 10.1103/PhysRevLett.122.107801.

Abstract

An achiral, bent-core mesogen forms several tilted smectic liquid crystal phases, including a nonpolar, achiral de Vries smectic A which transitions to a chiral, ferroelectric state in applied electric fields above a threshold. At lower temperature, a chiral, ferrielectric phase with a periodic, supermolecular modulation of the tilt azimuth, indicated by a Bragg peak in carbon-edge resonant soft x-ray scattering, is observed. The absence of a corresponding resonant umklapp peak identifies the superlayer structure as a twist-bend-like helix that is only weakly modulated by the smectic layering.