Tunable microsecond dynamics of an allosteric switch regulate the activity of a AAA+ disaggregation machine

Nat Commun. 2019 Mar 29;10(1):1438. doi: 10.1038/s41467-019-09474-6.

Abstract

Large protein machines are tightly regulated through allosteric communication channels. Here we demonstrate the involvement of ultrafast conformational dynamics in allosteric regulation of ClpB, a hexameric AAA+ machine that rescues aggregated proteins. Each subunit of ClpB contains a unique coiled-coil structure, the middle domain (M domain), proposed as a control element that binds the co-chaperone DnaK. Using single-molecule FRET spectroscopy, we probe the M domain during the chaperone cycle and find it to jump on the microsecond time scale between two states, whose structures are determined. The M-domain jumps are much faster than the overall activity of ClpB, making it an effectively continuous, tunable switch. Indeed, a series of allosteric interactions are found to modulate the dynamics, including binding of nucleotides, DnaK and protein substrates. This mode of dynamic control enables fast cellular adaptation and may be a general mechanism for the regulation of cellular machineries.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Allosteric Regulation
  • Binding Sites
  • Endopeptidase Clp / chemistry
  • Endopeptidase Clp / metabolism*
  • Fluorescence Resonance Energy Transfer
  • HSP70 Heat-Shock Proteins / metabolism
  • Models, Molecular
  • Protein Aggregates*
  • Protein Domains
  • Substrate Specificity
  • Thermus thermophilus / enzymology*
  • Time Factors

Substances

  • HSP70 Heat-Shock Proteins
  • Protein Aggregates
  • Endopeptidase Clp