Apoptotic cell-mimicking gold nanocages loaded with LXR agonist for attenuating the progression of murine systemic lupus erythematosus

Biomaterials. 2019 Mar:197:380-392. doi: 10.1016/j.biomaterials.2019.01.034. Epub 2019 Jan 23.

Abstract

Systemic lupus erythematosus (SLE) constitutes an autoimmune disease characterized by the breakdown of tolerance to self-antigens, sustained production of pathogenic autoantibodies, and damage to multiple organs and tissues. Nanoparticle (NP)-based therapeutics have demonstrated efficacy in attenuating the progression of SLE. However, investigations of nano-drugs that address the crucial initiating factor in the pathogenesis of SLE; e.g., inefficient clearance of apoptotic cells by phagocytes and consequent accumulation of self-antigens, have seldom been reported. Here, an apoptotic cell-mimicking gold nanocage (AuNC)-based nano drug carrier capable of correcting the impaired clearance of apoptotic cells in SLE was rationally designed and generated by conjugating phosphatidylserine (PS) on the surface of liposome-coated AuNCs for liver X receptor (LXR) agonist T0901317 delivery. Notably, PS-lipos-AuNC@T0901317 could efficiently enhance apoptotic cell clearance by elevating the expression of Mer, one of the pivotal phagocytosis-associated receptors on macrophages, resulting in decreased production of anti-dsDNA autoantibodies, reduced inflammatory response, and alleviation of kidney damage in lupus model mice. Additionally, PS-lipos-AuNC could be tracked by photoacoustic imaging for nano drug carrier biodistribution. By addressing the crucial pathogenic factor of SLE, the NP-based delivery system in this study is envisioned to provide a promising strategy to treat this complex and challenging disease.

Keywords: Apoptotic cell; Gold nanocage; Liver X receptor agonist; Phosphatidylserine; Systemic lupus erythematosus.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Apoptosis*
  • Autoantibodies / analysis
  • Cytokines / metabolism
  • Disease Progression
  • Drug Delivery Systems*
  • Drug Evaluation, Preclinical
  • Female
  • Gold / administration & dosage*
  • Gold / pharmacokinetics
  • Hydrocarbons, Fluorinated / administration & dosage*
  • Hydrocarbons, Fluorinated / therapeutic use
  • Hydrocarbons, Fluorinated / toxicity
  • Liposomes / administration & dosage
  • Liver X Receptors / agonists*
  • Lupus Erythematosus, Systemic / drug therapy*
  • Lupus Nephritis / drug therapy
  • Lupus Nephritis / immunology
  • Mice
  • Mice, Inbred C57BL
  • Mice, Inbred MRL lpr
  • Nanocapsules / administration & dosage*
  • Phosphatidylserines
  • Sulfonamides / administration & dosage*
  • Sulfonamides / therapeutic use
  • Sulfonamides / toxicity
  • Tissue Distribution
  • c-Mer Tyrosine Kinase / biosynthesis
  • c-Mer Tyrosine Kinase / genetics

Substances

  • Autoantibodies
  • Cytokines
  • Hydrocarbons, Fluorinated
  • Liposomes
  • Liver X Receptors
  • Nanocapsules
  • Phosphatidylserines
  • Sulfonamides
  • T0901317
  • Gold
  • Mertk protein, mouse
  • c-Mer Tyrosine Kinase