Mass spectrometry characterization for N-glycosylation of immunoglobulin Y from hen egg yolk

Int J Biol Macromol. 2018 Mar:108:277-283. doi: 10.1016/j.ijbiomac.2017.12.012. Epub 2017 Dec 5.

Abstract

Immunoglobulin Y (IgY) is a new therapeutic antibody that exists in hen egg yolk. It is a glycoprotein, not much is known about its N-glycan structures, site occupancy and site-specific N-glycosylation. In this study, purified protein from hen egg yolk was identified as IgY based on SDS-PAGE and MALDI-TOF/TOF MS. N-glycan was released from IgY using peptide-N4-(N-acetyl-beta-glucosaminyl) asparagine-amidase treatment, and the molecular weight of IgY was calculated using the difference between the molecular weight of IgY and deglycosylated IgY. Two potential N-Glycosylation sites (ASN308 and ASN409) were detected on IgY by nanoLC-ESI MS. Sugar chains were separated using normal phase liquid chromatography after fluorescence labeling, and 17 N-glycan structures were confirmed using ESI-MS. The sugar chain pattern contained high-mannose oligosaccharide, hybrid oligosaccharide and complex oligosaccharide. These results could lead to other important information regarding IgY glycosylation.

Keywords: Glycosylation; Immunoglobulin Y; N-glycan.

MeSH terms

  • Animals
  • Chickens
  • Chromatography, High Pressure Liquid
  • Egg Yolk / chemistry*
  • Glycoproteins / chemistry*
  • Glycoproteins / metabolism
  • Glycosylation
  • Immunoglobulins / chemistry*
  • Immunoglobulins / isolation & purification
  • Immunoglobulins / metabolism
  • Mass Spectrometry*
  • Molecular Weight
  • Polysaccharides / chemistry
  • Spectrometry, Mass, Matrix-Assisted Laser Desorption-Ionization

Substances

  • Glycoproteins
  • IgY
  • Immunoglobulins
  • Polysaccharides