Alternating 5,5-Dimethylcyclopentadiene and Diketopyrrolopyrrole Copolymer Prepared at Room Temperature for High Performance Organic Thin-Film Transistors

J Am Chem Soc. 2017 Jun 21;139(24):8094-8097. doi: 10.1021/jacs.7b03279. Epub 2017 Jun 12.

Abstract

We report that the inclusion of nonaromatic 5,5-dimethylcyclopentadiene monomer into a conjugated backbone is an attractive strategy to high performance semiconducting polymers. The use of this monomer enables a room temperature Suzuki copolymerization with a diketopyrrolopyrrole comonomer to afford a highly soluble, high molecular weight material. The resulting low band gap polymer exhibits excellent photo and thermal stability, and despite a large π-π stacking distance of 4.26 Å, it demonstrates excellent performance in thin-film transistor devices.

Publication types

  • Research Support, Non-U.S. Gov't

Associated data

  • figshare/10.6084/m9.figshare.5071846