Artemisia umbelliformis Lam. and Génépi Liqueur: Volatile Profile as Diagnostic Marker for Geographic Origin and To Predict Liqueur Safety

J Agric Food Chem. 2017 Apr 5;65(13):2849-2856. doi: 10.1021/acs.jafc.6b03394. Epub 2017 Mar 23.

Abstract

Artemisia umbelliformis, commonly known as "white génépi", is characterized by a volatile fraction rich in α- and β-thujones, two monoterpenoids; under European Union (EU) regulations these are limited to 35 mg/L in Artemisia-based beverages because of their recognized activity on the human central nervous system. This study reports the results of an investigation to define the geographical origin and thujone content of individual plants of A. umbelliformis from different geographical sites, cultivated experimentally at a single site, and to predict the thujone content in the resulting liqueurs through their volatile fraction. Headspace solid phase microextraction (HS-SPME) combined with gas chromatography-mass spectrometry (GC-MS) and non-separative HS-SPME-MS were used as analytical platforms to create a database suitable for chemometric description and prediction through linear discriminant analysis (LDA). HS-SPME-MS was applied to shorten analysis time. With both approaches, a diagnostic prediction of (i) plant geographical origin and (ii) thujone content of plant-related liqueurs could be made.

Keywords: Artemisia umbelliformis Lam.; food safety; génépi liqueur.

MeSH terms

  • Alcoholic Beverages / analysis*
  • Artemisia / chemistry*
  • Discriminant Analysis
  • Gas Chromatography-Mass Spectrometry
  • Geography
  • Solid Phase Microextraction
  • Volatile Organic Compounds / chemistry*

Substances

  • Volatile Organic Compounds