Long-term continuous production of H2 in a microbial electrolysis cell (MEC) treating saline wastewater

Water Res. 2015 Sep 15:81:149-56. doi: 10.1016/j.watres.2015.05.041. Epub 2015 Jun 5.

Abstract

A biofilm-based 4 L two chamber microbial electrolysis cell (MEC) was continuously fed with acetate under saline conditions (35 g/L NaCl) for more than 100 days. The MEC produced a biogas highly enriched in H2 (≥90%). Both current (10.6 ± 0.2 A/m(2)Anode or 199.1 ± 4.0 A/m(3)MEC) and H2 production (201.1 ± 7.5 LH2/m(2)Cathode·d or 0.9 ± 0.0 m(3)H2/m(3)MEC·d) rates were highly significant when considering the saline operating conditions. A microbial analysis revealed an important enrichment in the anodic biofilm with five main bacterial groups: 44% Proteobacteria, 32% Bacteroidetes, 18% Firmicutes and 5% Spirochaetes and 1% Actinobacteria. Of special interest is the emergence within the Proteobacteria phylum of the recently described halophilic anode-respiring bacteria Geoalkalibacter (unk. species), with a relative abundance up to 14%. These results provide for the first time a noteworthy alternative for the treatment of saline effluents and continuous production of H2.

Keywords: Biohydrogen; Geoalkalibacter; High-throughput sequencing; Microbial electrolysis cell; Saline wastewater; Scanning electron microscopy.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acetates / metabolism
  • Bacteria / metabolism*
  • Bioelectric Energy Sources*
  • Biofilms
  • Deltaproteobacteria / metabolism
  • Electrolysis / instrumentation
  • Hydrogen / metabolism*
  • Salinity
  • Waste Disposal, Fluid / methods
  • Wastewater / chemistry*

Substances

  • Acetates
  • Waste Water
  • Hydrogen