Sonochemical fabrication of dual-targeted redox-responsive smart microcarriers

ACS Appl Mater Interfaces. 2014 Dec 24;6(24):22166-73. doi: 10.1021/am5057097. Epub 2014 Dec 5.

Abstract

In the present study, the molecular and magnetic dual-targeted redox-responsive folic acid-cysteine-Fe3O4 microcapsules (FA-Cys-Fe3O4 MCs) have been synthesized via the sonochemical technique, and targeting molecule (folic acid) and Fe3O4 magnetic nanoparticles are introduced into the microcapsule shells successfully. The obtained FA-Cys-Fe3O4 MCs show excellent magnetic responsive ability by the oriented motion under an external magnetic field. The hydrophobic fluorescent dye (Coumarin 6) is successfully loaded into the FA-Cys-Fe3O4 MCs, demonstrating that it could be also easily realized to encapsulate hydrophobic drugs into the FA-Cys-Fe3O4 MCs when the drugs are dispersed into the oil phase before sonication. Cellular uptake demonstrates that FA-Cys-Fe3O4 MCs could target selectively the cells via folate-receptor-mediated endocytosis. Moreover, the FA-Cys-Fe3O4 MCs show their potential ability to be an attractive carrier for drug controlled release owing to the redox responsiveness of the disulfide in the microcapsule shells.

Keywords: dual-targeted; microcapsule; redox-responsive; sonochemical.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Capsules / chemical synthesis*
  • Capsules / radiation effects
  • Cysteine / chemistry
  • Delayed-Action Preparations / chemical synthesis*
  • Diffusion
  • Drug Compounding / methods
  • Folic Acid / administration & dosage*
  • Folic Acid / chemistry
  • HeLa Cells
  • High-Energy Shock Waves
  • Humans
  • Magnetite Nanoparticles / administration & dosage
  • Magnetite Nanoparticles / chemistry*
  • Magnetite Nanoparticles / ultrastructure
  • Materials Testing
  • Oxidation-Reduction / radiation effects
  • Particle Size
  • Sonication / methods*

Substances

  • Capsules
  • Delayed-Action Preparations
  • Magnetite Nanoparticles
  • Folic Acid
  • Cysteine