Potent inhibition of TGF-β signaling pathway regulator Abl: potential therapeutics for hepatic fibrosis

J Recept Signal Transduct Res. 2015;35(5):410-9. doi: 10.3109/10799893.2014.986745. Epub 2014 Nov 24.

Abstract

Hepatic fibrosis is overly exuberant wound healing in which excessive connective tissue builds up in the liver. The treatment of hepatic fibrosis is still difficult and remains a challenge to the clinician. In recent years, the TGF-β signaling pathway regulator tyrosine kinase Abl has been raised as a new and promising target of hepatic fibrosis therapy. Here, considering that there are numerous drugs and drug-like compounds being approved or under clinical development and experimental investigation, it is expected that some of the existing drugs can be re-exploited as new agents to target Abl with the capability of suppressing hepatic fibrosis. To achieve this, a synthetic protocol that integrated molecular docking, affinity scoring dynamics simulation and free energy analysis was described to systematically profile the inhibitory potency of various drugs and drug-like compounds against the kinase domain of Abl. Consequently, 4 out of 13 tested drug candidates were successfully identified to have high-Abl inhibitory activities. By visually examining the dynamics behavior, structural basis and energetic property of few typical Abl-drug complex cases, a significantly different pattern of non-bonded interactions between the binding of active and inactive drug ligands to Abl receptor was revealed; the former is defined by strong, specific chemical forces, while the latter can only form non-specific hydrophobic contacts with slight atomic collisions.

Keywords: Abl kinase; TGF-β signaling pathway; hepatic fibrosis.

MeSH terms

  • Binding Sites
  • Drug Design*
  • Drug Evaluation, Preclinical / methods
  • Enzyme Activation
  • Enzyme Inhibitors / chemistry*
  • Humans
  • Liver Cirrhosis / metabolism
  • Liver Cirrhosis / prevention & control
  • Models, Chemical
  • Molecular Docking Simulation*
  • Protein Binding
  • Protein Conformation
  • Proto-Oncogene Proteins c-abl / antagonists & inhibitors
  • Proto-Oncogene Proteins c-abl / chemistry*
  • Proto-Oncogene Proteins c-abl / ultrastructure*
  • Transforming Growth Factor beta / chemistry

Substances

  • Enzyme Inhibitors
  • Transforming Growth Factor beta
  • Proto-Oncogene Proteins c-abl