Human whole-blood (1)H2O longitudinal relaxation with normal and high-relaxivity contrast reagents: influence of trans-cell-membrane water exchange

Magn Reson Med. 2014 Dec;72(6):1746-54. doi: 10.1002/mrm.25064. Epub 2013 Dec 19.

Abstract

Purpose: Accurate characterization of contrast reagent (CR) longitudinal relaxivity in whole blood is required to predict arterial signal intensity in contrast-enhanced MR angiography (CE-MRA). This study measured the longitudinal relaxation rate constants (R1 ) over a concentration range for non-protein-binding and protein-binding CRs in ex vivo whole blood and plasma at 1.5 and 3.0 Tesla (T) under physiologic arterial conditions.

Methods: Relaxivities of gadoteridol, gadobutrol, gadobenate, and gadofosveset were measured for [CR] from 0 to 18 mM [mmol(CR)/L(blood)]: the latter being the upper limit of what may be expected in CE-MRA.

Results: In plasma, the (1) H2 O R1 [CR]-dependence was nonlinear for gadobenate and gadofosveset secondary to CR interactions with the serum macromolecule albumin, and was well described by an analytical expression for effective 1:1 binding stoichiometry. In whole blood, the (1) H2 O R1 [CR]-dependence was markedly non-linear for all CRs, and was well-predicted by an expression for equilibrium exchange of water molecules between plasma and intracellular spaces using a priori parameter values only.

Conclusion: In whole blood, (1) H2 O R1 exhibits a nonlinear relationship with [CR] over 0 to 18 mM CR. The nonlinearity is well described by exchange of water between erythrocyte and plasma compartments, and is particularly evident for high relaxivity CRs.

Keywords: MR angiography; MRI; contrast agents; relaxation rate constant; relaxation time constant.

Publication types

  • Comparative Study
  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Blood Chemical Analysis / methods*
  • Blood Proteins / chemistry*
  • Blood Proteins / radiation effects
  • Cell Membrane / chemistry*
  • Contrast Media / chemistry*
  • Contrast Media / radiation effects
  • Electric Impedance
  • Gadolinium / chemistry*
  • Gadolinium / radiation effects
  • Humans
  • Magnetic Fields
  • Magnetic Resonance Imaging / methods*
  • Protons
  • Radiation Dosage
  • Water / chemistry*

Substances

  • Blood Proteins
  • Contrast Media
  • Protons
  • Water
  • Gadolinium