The rigid amphipathic fusion inhibitor dUY11 acts through photosensitization of viruses

J Virol. 2014 Feb;88(3):1849-53. doi: 10.1128/JVI.02907-13. Epub 2013 Nov 27.

Abstract

Rigid amphipathic fusion inhibitors (RAFIs) are lipophilic inverted-cone-shaped molecules thought to antagonize the membrane curvature transitions that occur during virus-cell fusion and are broad-spectrum antivirals against enveloped viruses (Broad-SAVE). Here, we show that RAFIs act like membrane-binding photosensitizers: their antiviral effect is dependent on light and the generation of singlet oxygen ((1)O(2)), similar to the mechanistic paradigm established for LJ001, a chemically unrelated class of Broad-SAVE. Photosensitization of viral membranes is a common mechanism that underlies these Broad-SAVE.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antiviral Agents / chemistry
  • Antiviral Agents / pharmacology*
  • Cell Membrane / drug effects*
  • Cell Membrane / radiation effects
  • Cell Membrane / virology
  • Herpes Simplex / virology*
  • Herpesvirus 1, Human / drug effects*
  • Herpesvirus 1, Human / genetics
  • Herpesvirus 1, Human / physiology
  • Herpesvirus 1, Human / radiation effects
  • Humans
  • Light
  • Virus Internalization / drug effects*

Substances

  • Antiviral Agents