Selective hydrothermal method to create patterned and photoelectrochemically effective Pt/WO3 interfaces

ACS Appl Mater Interfaces. 2013 Dec 26;5(24):13050-4. doi: 10.1021/am4039536. Epub 2013 Dec 10.

Abstract

A hydrothermal method based on the use of hydrogen peroxide is described to grow a homogeneous layer of tungsten oxide (WO3) on a platinum (Pt) film supported on a silicon wafer. WO3 growth is highly selective for Pt when present on silicon in a patterned arrangement, demonstrating that Pt catalyzes decomposition of the WO3 precursor in solution. The obtained Pt/WO3 interface yields high photocurrents of 1.1 mA/cm(2) in photoelectrochemical water splitting when illuminated by a solar simulator. The photocurrents are significantly higher than most previously reported values for hydrothermally grown layers on indium-tin oxide and fluorine-tin oxide glasses. The selective growth method thus provides new options to effectively implement WO3 in photoelectrochemical devices.

Publication types

  • Research Support, Non-U.S. Gov't