Neuroprotection by monocarbonyl dimethoxycurcumin C: ameliorating the toxicity of mutant TDP-43 via HO-1

Mol Neurobiol. 2014 Feb;49(1):368-79. doi: 10.1007/s12035-013-8525-4. Epub 2013 Aug 10.

Abstract

Mutation of TAR DNA-binding protein-43 (TDP-43) was detected in familiar and sporadic amyotrophic lateral sclerosis, and pathological TDP-43 was identified in the frontotemporal lobar degeneration. The neuroprotective functions of curcumin derivatives were assessed in motor neurons transfected with mutant TDP-43. We found that curcumin derivatives reduced the levels of TDP-43 fragments. Furthermore, we evaluated these compounds on the cellular model that the cells were transfected with TDP-25. We found that the expression level and aggregate formation of TDP-25 were significantly reduced by monocarbonyl dimethoxycurcumin C (Compound C). To study on the neuroprotective functions of curcumin derivatives, the neuroblastoma-spinal cord-34 cells transfected with mutant TDP-43 were assessed by the level of lactate dehydrogenase (LDH) and malondialdehyde bisdimethyl acetal (MDA) that were involved in the oxidative stress. We found that Compound C ameliorated the damage of mutant TDP-43 by reducing the level of MDA and LDH. Furthermore, heme oxygenase-1 (HO-1) was induced by Compound C significantly higher than other compounds. Znpp, which is known an inhibitor of HO-1, dramatically interfered with the function of Compound C. In addition, Compound C was tested in vivo, and HO-1 was significantly upregulated at the hippocampus. These findings suggest that Compound C, which degrades TDP-43 fragment and strengthens the antioxidant ability by HO-1, is a promising agent for TDP-43 proteinopathy.

MeSH terms

  • Animals
  • Cell Line
  • Curcumin / analogs & derivatives*
  • Curcumin / pharmacology
  • DNA-Binding Proteins / antagonists & inhibitors
  • DNA-Binding Proteins / genetics*
  • DNA-Binding Proteins / metabolism*
  • Dose-Response Relationship, Drug
  • Heme Oxygenase-1 / biosynthesis*
  • Humans
  • Male
  • Membrane Proteins / biosynthesis*
  • Mice
  • Mice, Inbred C57BL
  • Mutation / genetics*
  • Neuroprotective Agents / pharmacology*
  • Oxidative Stress / drug effects
  • Oxidative Stress / physiology

Substances

  • DNA-Binding Proteins
  • Membrane Proteins
  • Neuroprotective Agents
  • TDP-43 protein, mouse
  • dimethoxycurcumin
  • Heme Oxygenase-1
  • Hmox1 protein, mouse
  • Curcumin