Phosphaalkene vs. phosphinidene: the nature of the P-C bond in carbonyl-decorated carbene → PPh adducts

Chem Commun (Camb). 2014 Jan 7;50(2):162-4. doi: 10.1039/c3cc45134h.

Abstract

Treatment of dichlorophenylphosphine with two equivalents of carbonyl-decorated carbenes results in a two-electron reduction of the phosphorus centre concomitant with carbene oxidation to afford novel phosphaalkenes as confirmed via crystallographic, spectroscopic, and DFT analyses.