Bias-enhanced optical pH response of group III-nitride nanowires

Nano Lett. 2012 Dec 12;12(12):6180-6. doi: 10.1021/nl303021v. Epub 2012 Nov 12.

Abstract

We show that the photoluminescence intensity of GaN and InGaN nanowires in electrolytes sensitively responds to variations of the pH value and the applied bias. The realization of an electrochemical working point allows pH detection with a resolution better than 0.05 pH. The observed effects are attributed to bias-dependent nonradiative recombination processes competing with interband transitions. The results show that group III-nitride nanowires are excellently suited as nanophotonic pH sensor elements.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Electrochemical Techniques
  • Electrolytes / chemistry
  • Gallium / chemistry*
  • Hydrogen-Ion Concentration
  • Indium / chemistry*
  • Luminescence
  • Nanowires / chemistry*

Substances

  • Electrolytes
  • Indium
  • gallium nitride
  • Gallium