σ-Donor-σ-acceptor plumbylene ligands: synergic σ-donation between ambiphilic Pt(0) and Pb(II) fragments

Chem Commun (Camb). 2012 Oct 28;48(84):10410-2. doi: 10.1039/c2cc35777a. Epub 2012 Sep 19.

Abstract

Mono- and diplatinum plumbylene complexes are prepared in which the bonding comprises synergic σ donation between the Pt and Pb atoms. The bonding distinguishes the complexes from both the classical Fischer carbene bonding model and M→Pb dative-only bonding. The Pt-Pb bond of the monoplatinum complex is stable, while the diplatinum complex reversibly loses one Pt fragment.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Lead / chemistry*
  • Ligands
  • Models, Molecular
  • Molecular Structure
  • Organometallic Compounds / chemical synthesis
  • Organometallic Compounds / chemistry*
  • Organophosphorus Compounds / chemistry*
  • Platinum / chemistry*

Substances

  • Ligands
  • Organometallic Compounds
  • Organophosphorus Compounds
  • Lead
  • Platinum