Stereoselective synthesis and antiviral activity of methyl-substituted cycloSal-pronucleotides

J Med Chem. 2012 Aug 23;55(16):7245-52. doi: 10.1021/jm3008085. Epub 2012 Aug 3.

Abstract

Methyl-substituted cycloSal-pronucleotides of d4TMP were synthesized with high diastereoselectivities in satisfying chemical yields. The individual diastereomers were tested against HIV-1 and HIV-2 infected wild-type CEM/0 and HIV-2 infected thymidine kinase deficient CEM cells. All diastereomers tested showed significant antiviral activity in CEM/0 and strong activity in CEM/TK(-) cell cultures. The antiviral activities were strongly dependent on the chirality at the phosphate group and the position of the methyl-group(s) in the cycloSal moiety. In CEM/TK(-) cell cultures the difference in antiviral potency was found to be 7- to 20-fold. The stability of each diastereomer was studied in aqueous phosphate buffer and in CEM/0 cell extracts. Large differences in the half-lives were found. A comparison of the relative lipophilicity of the methyl-substituted cycloSal triesters was performed based on the retention times obtained by reversed phase HPLC. The results obtained clearly confirm the importance of a diastereoselective synthesis of cycloSal-pronucleotides.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Anti-HIV Agents / chemical synthesis*
  • Anti-HIV Agents / chemistry
  • Anti-HIV Agents / pharmacology
  • Cell Line
  • Dideoxynucleotides / chemical synthesis*
  • Dideoxynucleotides / chemistry
  • Dideoxynucleotides / pharmacology
  • Drug Stability
  • HIV-1 / drug effects
  • HIV-2 / drug effects
  • Humans
  • Hydrolysis
  • Mutation
  • Solvents / chemistry
  • Stavudine / analogs & derivatives*
  • Stavudine / chemical synthesis
  • Stavudine / chemistry
  • Stavudine / pharmacology
  • Stereoisomerism
  • Structure-Activity Relationship
  • Thymidine Kinase / genetics
  • Thymine Nucleotides / chemical synthesis*
  • Thymine Nucleotides / chemistry
  • Thymine Nucleotides / pharmacology

Substances

  • Anti-HIV Agents
  • Cyclosaligenyl-2',3'-didehydro-2',3'-dideoxythymidine monophosphate
  • Dideoxynucleotides
  • Solvents
  • Thymine Nucleotides
  • Stavudine
  • Thymidine Kinase