Stable-isotope dilution GC-MS method for ethanol in vapour ethanol and microdialysis systems based on carbonate-catalyzed extractive pentafluorobenzoylation

Analyst. 2012 May 21;137(10):2480-5. doi: 10.1039/c2an16135d. Epub 2012 Mar 27.

Abstract

Common ethanol detection methods are not applicable to cell culture media and microdialysates due to interference with medium constituents including amino acids and pH indicators. We present a novel GC-MS method for the accurate and precise analysis of ethanol in cell cultures and microdialysates. The method is based on the carbonate-catalyzed extractive pentafluorobenzoylation of ethanol and deuterium-labelled ethanol serving as the internal standard and on their GC-MS analysis in the electron-capture negative-ion chemical ionization mode. The method was used to optimize experimental conditions in a custom-made ethanol vapour system utilized for studies examining ethanol influences on neuronal cell lines and in microdialysis.

MeSH terms

  • Amino Acids / chemistry
  • Benzoates / chemistry*
  • Carbonates / chemistry*
  • Catalysis
  • Cell Line, Tumor
  • Deuterium / chemistry
  • Ethanol / analysis*
  • Gas Chromatography-Mass Spectrometry*
  • Gases / analysis*
  • Humans
  • Hydrogen-Ion Concentration
  • Microdialysis
  • Radioisotope Dilution Technique

Substances

  • Amino Acids
  • Benzoates
  • Carbonates
  • Gases
  • pentafluorobenzoyl chloride
  • Ethanol
  • Deuterium