Improved oral bioavailability of poorly water-soluble indirubin by a supersaturatable self-microemulsifying drug delivery system

Int J Nanomedicine. 2012:7:1115-25. doi: 10.2147/IJN.S28761. Epub 2012 Feb 23.

Abstract

Background: Indirubin, isolated from the leaves of the Chinese herb Isatis tinctoria L, is a protein kinase inhibitor and promising antitumor agent. However, the poor water solubility of indirubin has limited its application. In this study, a supersaturatable self-microemulsifying drug delivery system (S-SMEDDS) was developed to improve the oral bioavailability of indirubin.

Methods: A prototype S-SMEDDS was designed using solubility studies and phase diagram construction. Precipitation inhibitors were selected from hydrophilic polymers according to their crystallization-inhibiting capacity through in vitro precipitation tests. In vitro release of indirubin from S-SMEDDS was examined to investigate its likely release behavior in vivo. The in vivo bioavailability of indirubin from S-SMEDDS and from SMEDDS was compared in rats.

Results: The prototype formulation of S-SMEDDS comprised Maisine™ 35-1:Cremophor(®) EL:Transcutol(®) P (15:40:45, w/w/w). Polyvinylpyrrolidone K17, a hydrophilic polymer, was used as a precipitation inhibitor based on its better crystallization-inhibiting capacity compared with polyethylene glycol 4000 and hydroxypropyl methylcellulose. In vitro release analysis showed more rapid drug release from S-SMEDDS than from SMEDDS. In vivo bioavailability analysis in rats indicated that improved oral absorption was achieved and that the relative bioavailability of S-SMEDDS was 129.5% compared with SMEDDS.

Conclusion: The novel S-SMEDDS developed in this study increased the dissolution rate and improved the oral bioavailability of indirubin in rats. The results suggest that S-SMEDDS is a superior means of oral delivery of indirubin.

Keywords: bioavailability; hydrophilic polymer; indirubin; oral drug delivery; supersaturatable self-microemulsifying drug delivery system.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Administration, Oral
  • Analysis of Variance
  • Animals
  • Area Under Curve
  • Biological Availability
  • Drug Delivery Systems*
  • Emulsifying Agents / chemistry*
  • Emulsions / administration & dosage
  • Emulsions / chemistry
  • Emulsions / pharmacokinetics
  • Hydrophobic and Hydrophilic Interactions
  • Hypromellose Derivatives
  • Indoles / administration & dosage
  • Indoles / chemistry
  • Indoles / pharmacokinetics
  • Methylcellulose / analogs & derivatives
  • Methylcellulose / chemistry
  • Polyethylene Glycols / chemistry
  • Povidone / chemistry
  • Rats
  • Rats, Sprague-Dawley
  • Solubility

Substances

  • Emulsifying Agents
  • Emulsions
  • Indoles
  • Hypromellose Derivatives
  • Polyethylene Glycols
  • Methylcellulose
  • Povidone
  • indirubin