Self-assembled polymersomes conjugated with lactoferrin as novel drug carrier for brain delivery

Pharm Res. 2012 Jan;29(1):83-96. doi: 10.1007/s11095-011-0513-7. Epub 2011 Oct 7.

Abstract

Purpose: To develop a novel brain drug delivery system based on self-assembled poly(ethyleneglycol)-poly (D,L-lactic-co-glycolic acid) (PEG-PLGA) polymersomes conjugated with lactoferrin (Lf-POS). The brain delivery properties of Lf-POS were investigated and optimized.

Method: Three formulations of Lf-POS, with different densities of lactoferrin on the surface of polymersomes, were prepared and characterized. The brain delivery properties in mice were investigated using 6-coumarin as a fluorescent probe loaded in Lf-POS (6-coumarin-Lf-POS). A neuroprotective peptide, S14G-humanin, was incorporated into Lf-POS (SHN-Lf-POS); a protective effect on the hippocampuses of rats treated by Amyloid-β(25-35) was investigated by immunohistochemical analysis.

Results: The results of brain delivery in mice demonstrated that the optimized number of lactoferrin conjugated per polymersome was 101. This obtains the greatest blood-brain barrier (BBB) permeability surface area(PS) product and percentage of injected dose per gram brain (%ID/g brain). Immunohistochemistry revealed the SHN-Lf-POS had a protective effect on neurons of rats by attenuating the expression of Bax and caspase-3 positive cells. Meanwhile, the activity of choline acetyltransferase (ChAT) had been increased compared with negative controls.

Conclusion: These results suggest that lactoferrin functionalized self-assembled PEG-PLGA polymersomes could be a promising brain-targeting peptide drug delivery system via intravenous administration.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alzheimer Disease / drug therapy
  • Animals
  • Blood-Brain Barrier / metabolism*
  • Caspase 3 / analysis
  • Coumarins / analysis
  • Cryoelectron Microscopy
  • Drug Carriers / chemistry
  • Drug Carriers / pharmacokinetics*
  • Lactic Acid / chemistry
  • Lactic Acid / pharmacokinetics*
  • Lactoferrin / chemistry
  • Lactoferrin / pharmacokinetics*
  • Liposomes
  • Male
  • Mice
  • Mice, Inbred BALB C
  • Particle Size
  • Peptides / chemistry
  • Peptides / pharmacokinetics
  • Polyethylene Glycols / chemistry
  • Polyethylene Glycols / pharmacokinetics
  • Polyglycolic Acid / chemistry
  • Polyglycolic Acid / pharmacokinetics*
  • Polylactic Acid-Polyglycolic Acid Copolymer
  • Rats
  • Rats, Sprague-Dawley
  • Surface Properties
  • Thiazoles / analysis
  • Tissue Distribution / drug effects

Substances

  • Coumarins
  • Drug Carriers
  • Gly(14)-Humanin
  • Liposomes
  • Peptides
  • Thiazoles
  • coumarin 6
  • Polylactic Acid-Polyglycolic Acid Copolymer
  • Polyglycolic Acid
  • Lactic Acid
  • Polyethylene Glycols
  • Lactoferrin
  • Caspase 3