Ionic liquid-based homogeneous liquid-liquid microextraction for the determination of antibiotics in milk by high-performance liquid chromatography

J Chromatogr A. 2011 Oct 14;1218(41):7254-63. doi: 10.1016/j.chroma.2011.08.063. Epub 2011 Aug 25.

Abstract

Ionic liquid-based homogeneous liquid-liquid microextraction (IL-based HLLME) high-performance liquid chromatography was developed and applied to the extraction, separation and determination of some antibiotics in milk. The proteins and lipids were removed by adding salt and adjusting the pH value. The homogeneous extraction was applied to the improvement of recoveries for IL phase and analytes. The experimental parameters of the IL-based HLLME, including salt concentration in sample solution, pH value of sample solution, volume of [C(6)MIM][BF(4)], amount of ion-pairing agent (NH(4)PF(6)), and extraction time, were evaluated. The limits of detection for enoxacin, pefloxacin, norfloxacin, enrofloxacin, sulfamethoxazole and sulfadimethoxine were 15.8, 7.07, 5.13, 4.00, 7.79 and 8.33 μg L(-1), respectively. When the proposed method was applied to the analysis of milk samples the recoveries of the analytes ranged from 92.5 to 118.6% and relative standard deviations were lower than 7.00%.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Anti-Bacterial Agents / analysis*
  • Anti-Bacterial Agents / isolation & purification
  • Chromatography, High Pressure Liquid / methods*
  • Drug Residues / analysis*
  • Drug Residues / isolation & purification
  • Fluoroquinolones / analysis
  • Fluoroquinolones / isolation & purification
  • Hydrogen-Ion Concentration
  • Ionic Liquids / chemistry
  • Liquid Phase Microextraction / methods*
  • Milk / chemistry*
  • Phosphoric Acids / chemistry
  • Sensitivity and Specificity
  • Sodium Chloride / chemistry
  • Sulfonamides / analysis
  • Sulfonamides / isolation & purification

Substances

  • Anti-Bacterial Agents
  • Fluoroquinolones
  • Ionic Liquids
  • Phosphoric Acids
  • Sulfonamides
  • Sodium Chloride
  • ammonium hexafluorophosphate