Identification of potassium dehydroandrographolidi succinas and its major metabolites in rat urine by liquid chromatography-tandem mass spectrometry

J Chromatogr B Analyt Technol Biomed Life Sci. 2011 Jul 15;879(22):2107-12. doi: 10.1016/j.jchromb.2011.05.046. Epub 2011 Jun 12.

Abstract

A rapid, sensitive and specific liquid chromatography-tandem mass spectrometry (LC-MS/MS) method has been developed for identification of potassium dehydroandrographolidi succinas and its metabolites in rat urine. Five male rats were administrated a single dose (100 mg/kg) of potassium dehydroandrographolidi succinas by i.v. injection. The urine were sampled from 0 to 24 h and purified by using Oasis® HLB extraction cartridge, then the purified urine samples were separated on a reversed-phase C18 column with a linear gradient and detected by an on-line MS detector. Identification and structural elucidation of the metabolites were performed by comparing their changes in molecular mass (Δm) and MS/MS spectra with those of the parent drug. Seven metabolites and the parent drug were found in rat urine. All these metabolites were reported for the first time.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Andrographis / chemistry*
  • Animals
  • Chromatography, Reverse-Phase / methods*
  • Diterpenes / chemistry
  • Diterpenes / isolation & purification
  • Diterpenes / metabolism
  • Diterpenes / urine*
  • Drugs, Chinese Herbal
  • Male
  • Metabolic Networks and Pathways
  • Rats
  • Rats, Wistar
  • Sensitivity and Specificity
  • Tandem Mass Spectrometry / methods*

Substances

  • Diterpenes
  • Drugs, Chinese Herbal
  • andrographolide