Small-molecule activators of AMP-activated protein kinase (AMPK), RSVA314 and RSVA405, inhibit adipogenesis

Mol Med. 2011 Sep-Oct;17(9-10):1022-30. doi: 10.2119/molmed.2011.00163. Epub 2011 Jun 1.

Abstract

AMP-activated protein kinase (AMPK) is a sensor and regulator of cellular energy metabolism potentially implicated in a broad range of conditions, including obesity and Alzheimer's disease. Its role in the control of key metabolic enzymes makes this kinase a central player in glucose and lipid homeostasis. Recently, by screening a library of synthetic small molecules selected for their structural similarity with the natural polyphenol resveratrol, we identified RSVA314 and RSVA405 as potent indirect activators of AMPK (half-maximal effective concentration [EC₅₀] = 1 μmol/L in cell-based assays). Here we show that RSVA314 and RSVA405 can significantly activate AMPK and inhibit acetyl-CoA carboxylase (ACC), one target of AMPK and a key regulator of fatty acid biogenesis, in nondifferentiated and proliferating 3T3-L1 adipocytes. We found that RSVA314 and RSVA405 treatments inhibited 3T3-L1 adipocyte differentiation by interfering with mitotic clonal expansion during preadipocyte proliferation (half-maximal inhibitory concentration [IC₅₀] = 0.5 μmol/L). RSVA314 and RSVA405 prevented the adipogenesis-dependent transcriptional changes of multiple gene products involved in the adipogenic process, including peroxisome proliferator-activated receptor (PPAR)-γ, CCAAT/enhancer-binding protein α (C/EBPα), fatty acid synthase, fatty acid binding protein 4 (aP2), RANTES or resistin. Furthermore, orally administered RSVA405 at 20 and 100 mg/kg/d significantly reduced the body weight gain of mice fed a high-fat diet. This work shows that the novel small-molecule activators of AMPK (RSVA314 and RSVA405) are potent inhibitors of adipogenesis and thus may have therapeutic potential against obesity.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • 3T3-L1 Cells
  • AMP-Activated Protein Kinases / metabolism*
  • Adipocytes / drug effects
  • Adipocytes / enzymology
  • Adipocytes / metabolism
  • Adipogenesis / drug effects*
  • Adipogenesis / genetics
  • Aminophenols / chemistry
  • Aminophenols / pharmacology*
  • Animals
  • Antioxidants / chemistry
  • Antioxidants / pharmacology
  • Blotting, Western
  • Body Weight / drug effects
  • CCAAT-Enhancer-Binding Protein-alpha / genetics
  • CCAAT-Enhancer-Binding Protein-alpha / metabolism
  • Cell Proliferation / drug effects
  • Dietary Fats / adverse effects
  • Enzyme Activation / drug effects
  • Enzyme Activators / chemistry
  • Enzyme Activators / pharmacology*
  • Fatty Acid Synthases / genetics
  • Fatty Acid Synthases / metabolism
  • Gene Expression / drug effects
  • Hydrazones / chemistry
  • Hydrazones / pharmacology*
  • Male
  • Mice
  • Mice, Inbred C57BL
  • Molecular Structure
  • Obesity / etiology
  • Obesity / prevention & control
  • PPAR gamma / genetics
  • PPAR gamma / metabolism
  • Resveratrol
  • Reverse Transcriptase Polymerase Chain Reaction
  • Stilbenes / chemistry
  • Stilbenes / pharmacology*
  • Weight Gain / drug effects

Substances

  • Aminophenols
  • Antioxidants
  • CCAAT-Enhancer-Binding Protein-alpha
  • Dietary Fats
  • Enzyme Activators
  • Hydrazones
  • PPAR gamma
  • RSVA314
  • RSVA405
  • Stilbenes
  • Fatty Acid Synthases
  • AMP-Activated Protein Kinases
  • Resveratrol