Antidiabetic sulfonylureas modulate farnesoid X receptor activation and target gene transcription

Future Med Chem. 2010 Apr;2(4):575-86. doi: 10.4155/fmc.10.10.

Abstract

Background: The sulfonylureas glibenclamide and glimepiride are oral antidiabetic drugs that stimulate insulin secretion by closing pancreatic ATP-dependent potassium channels. The farnesoid X receptor (FXR) is a ligand-activated transcription factor that regulates the expression of several target genes involved in bile acid metabolism and lipid and glucose homeostasis.

Methods: In this study we investigated the potential effects of sulfonylureas on the signaling of FXR using a reporter-gene assay, real-time qPCR and computational methods such as molecular docking and molecular dynamic simulations.

Results: We demonstrate that glibenclamide and glimepiride modulate FXR activation in a reporter-gene assay and induce FXR target genes in HepG2 cells. Within the docking experiments and molecular dynamics simulation, we found glibenclamide interacting with the ligand-binding domain of FXR and with helix 12.

Conclusion: Glibenclamide and glimepiride are potential ligands of FXR and modulate activation and signaling.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • COS Cells
  • Chlorocebus aethiops
  • Genes, Reporter
  • Glyburide / chemistry
  • Glyburide / metabolism
  • Glyburide / pharmacology
  • Hep G2 Cells
  • Humans
  • Hypoglycemic Agents / chemistry
  • Hypoglycemic Agents / metabolism
  • Hypoglycemic Agents / pharmacology*
  • Models, Molecular
  • Molecular Dynamics Simulation
  • Protein Conformation
  • Receptors, Cytoplasmic and Nuclear / chemistry
  • Receptors, Cytoplasmic and Nuclear / genetics
  • Receptors, Cytoplasmic and Nuclear / metabolism*
  • Signal Transduction / drug effects*
  • Sulfonylurea Compounds / chemistry
  • Sulfonylurea Compounds / metabolism
  • Sulfonylurea Compounds / pharmacology*
  • Transcriptional Activation / drug effects*

Substances

  • Hypoglycemic Agents
  • Receptors, Cytoplasmic and Nuclear
  • Sulfonylurea Compounds
  • farnesoid X-activated receptor
  • glimepiride
  • Glyburide