Efficient, global-scale quantification of absolute protein amounts by integration of targeted mass spectrometry and two-dimensional gel-based proteomics

Anal Chem. 2011 Apr 1;83(7):2677-84. doi: 10.1021/ac1031836. Epub 2011 Mar 11.

Abstract

Knowledge on absolute protein concentrations is mandatory for the simulation of biological processes in the context of systems biology. A novel approach for the absolute quantification of proteins at a global scale has been developed and its applicability demonstrated using glucose starvation of the Gram-positive model bacterium Bacillus subtilis and the pathogen Staphylococcus aureus as proof-of-principle examples. Absolute intracellular protein concentrations were initially determined for a preselected set of anchor proteins by employing a targeted mass spectrometric method and isotopically labeled internal standard peptides. Known concentrations of these anchor proteins were then used to calibrate two-dimensional (2-D) gels allowing the calculation of absolute abundance of all detectable proteins on the 2-D gels. Using this approach, concentrations of the majority of metabolic enzymes were determined, and thus a quantification of the players of metabolism was achieved. This new strategy is fast, cost-effective, applicable to any cell type, and thus of value for a broad community of laboratories with experience in 2-D gel-based proteomics and interest in quantitative approaches. Particularly, this approach could also be utilized to quantify existing data sets with the aid of a few standard anchor proteins.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Bacillus subtilis / cytology
  • Bacillus subtilis / metabolism
  • Bacterial Proteins / isolation & purification
  • Bacterial Proteins / metabolism
  • Cattle
  • Electrophoresis, Gel, Two-Dimensional / methods*
  • Humans
  • Mass Spectrometry / methods*
  • Proteins / isolation & purification*
  • Proteins / metabolism*
  • Proteomics / methods*
  • Staphylococcus aureus / cytology
  • Staphylococcus aureus / metabolism
  • Systems Integration*

Substances

  • Bacterial Proteins
  • Proteins