Evaluation of dioxin-like activities in settled house dust from Vietnamese E-waste recycling sites: relevance of polychlorinated/brominated dibenzo-p-dioxin/furans and dioxin-like PCBs

Environ Sci Technol. 2010 Dec 1;44(23):9195-200. doi: 10.1021/es102505j. Epub 2010 Nov 8.

Abstract

Few studies have investigated the human exposure to the ensemble of dioxin-related compounds (DRCs) released from uncontrolled e-waste recycling, especially from a toxic effect standpoint. This study evaluated the TCDD toxic equivalents (TEQs) in persistent extracts of settled house dust from two Vietnamese e-waste recycling sites (EWRSs) using the Dioxin-Responsive Chemically Activated LUciferase gene eXpression assay (DR-CALUX), combined with chemical analysis of PCDD/Fs, DL-PCBs, PBDD/Fs, and monobromo PCDD/Fs to determine their TEQ contribution. The CALUX-TEQ levels in house dust ranged from 370 to 1000 pg g(-1) in the EWRSs, approximately 3.5-fold higher than in the urban control site. In EWRS house dust, the concentrations of the unregulated PBDFs were 7.7-63 ng g(-1), an order of magnitude higher than those of regulated DRCs (PCDD/Fs and DL-PCBs), and PBDFs were also principal CALUX-TEQ contributors (4.2-22%), comparable to PCDD/Fs (8.1-29%). The CALUX-TEQ contribution of DRCs varied, possibly depending on thermal processing activities (higher PCDD/F-TEQs) and PBDE content in the waste (higher PBDF-TEQs). However, the percentage of unknown dioxin-like activities was high in all dust samples, indicating large contribution from unidentified DRCs and/or synergy among contaminants. Estimates of TEQ intake from dust ingestion suggest that children in the EWRSs may be adversely affected by DRCs from dust.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Benzofurans / analysis*
  • Benzofurans / toxicity
  • Dibenzofurans, Polychlorinated
  • Dioxins / analysis
  • Dioxins / toxicity
  • Dust / analysis
  • Electronic Waste / analysis*
  • Environmental Exposure / analysis
  • Environmental Monitoring
  • Environmental Pollutants / analysis*
  • Environmental Pollutants / toxicity
  • Humans
  • Polychlorinated Biphenyls / analysis*
  • Polychlorinated Biphenyls / toxicity
  • Polychlorinated Dibenzodioxins / analogs & derivatives*
  • Polychlorinated Dibenzodioxins / analysis
  • Polychlorinated Dibenzodioxins / toxicity
  • Vietnam
  • Waste Management / methods

Substances

  • Benzofurans
  • Dibenzofurans, Polychlorinated
  • Dioxins
  • Dust
  • Environmental Pollutants
  • Polychlorinated Dibenzodioxins
  • Polychlorinated Biphenyls