A new molybdenum(V) nickel phosphate based on divacant [H30(Mo(V)16O32)Ni14(PO4)26O2(OH)4(H2O)8]12- wheel

Dalton Trans. 2009 Nov 21:(43):9446-51. doi: 10.1039/b905277a. Epub 2009 Sep 17.

Abstract

A new molybdenum nickel phosphate, [H(2)en](3)Na(4)[Ni(H(2)O)(3)][H(30)(Mo(V)(16)O(32))Ni(14)(PO(4))(26)O(2) (OH)(4)(H(2)O)(8)] x 8 H(2)O 1, has been hydrothermally synthesized and structurally characterized. Compound 1 crystallizes in the monoclinic space group P2(1)/c with a = 18.6118(6) A, b = 20.9879(6) A, c = 22.9360(5) A, beta = 116.678(2) degrees, V = 8005.5(4) A(3) and Z = 2. The polyoxoanion of 1 exhibits an unusual divacant wheel-type cluster in which two {NiO(6)} octahedra are lost from the well-known "saturated" {Mo(16)TM(16)P(26)} wheel. The two vacant sites are occupied by two protonated ethylenediamines (H(2)en) via the strong hydrogen-bonding interactions between the surface O atoms of the polyoxoanions and the amine group derived from the H(2)en ligands. DC susceptibility measurements show that compound 1 exhibits strong antiferromagnetic interactions inside the wheel-type cluster.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Hydrogen Bonding
  • Magnetics
  • Models, Molecular
  • Molecular Conformation
  • Molybdenum / chemistry
  • Nickel / chemistry
  • Phosphates / chemical synthesis
  • Phosphates / chemistry*
  • Spectrophotometry, Infrared
  • Thermogravimetry
  • Tungsten Compounds / chemistry
  • Vanadium / chemistry

Substances

  • Phosphates
  • Tungsten Compounds
  • polyoxometalate I
  • Vanadium
  • Nickel
  • Molybdenum