Innermolecular reactions of fluorophenylcarbene inside a hemicarcerand

Org Lett. 2009 Sep 3;11(17):3866-9. doi: 10.1021/ol901474u.

Abstract

Photolysis of fluorophenyldiazirine, incarcerated in hemicarcerand 2, affords fluorophenylcarbene, which attacks an aryl unit of the host, leading (after rearrangement) to a fluoromethoxy/phenyltropone derivative of the hemicarcerand. The incarcerated carbene is probably unstable at temperatures above 100 K.