Ion-pairing high-performance liquid chromatography determination of amitrole in apple after solid-phase extraction and precolumn derivatization

Anal Bioanal Chem. 2009 Sep;395(2):465-71. doi: 10.1007/s00216-009-2962-y. Epub 2009 Jul 26.

Abstract

A novel method based on solid-phase extraction was studied for the extraction of amitrole (3-amino-1,2,4-triazole), and its residue determination in apples has been developed. The samples were derivatized with 4-chloro-3,5-dinitrobenzotrifluoride (CNBF). The derivatization conditions and the influence of elution composition on the separation were investigated. In pH 9.5 H(3)BO(3)-Na(2)B(4)O(7) media, the reaction of amitrole with CNBF was complete at 60 degrees C after 30 min. The separation of derivatized amitrole was achieved at room temperature within 13 min by gradient elution mode with cetyltrimethylammonium bromide in mobile phase as ion-pair reagent. The method correlation coefficient was 0.9996, in concentrations ranging from 1.66 to 415 mg L(-1). The calculated recoveries of the proposed method were from 94.17% to 105.67%, and relative standard deviations were 1.57% to 6.44% in the application to the quantitative determination of amitrole in apples. The detection limit of amitrole was 0.10 mg L(-1) with a signal-to-noise ratio of 3.

Publication types

  • Evaluation Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amitrole / analysis*
  • Chromatography, High Pressure Liquid / methods*
  • Fluorobenzenes
  • Herbicides / analysis*
  • Malus / chemistry*
  • Nitro Compounds
  • Sensitivity and Specificity
  • Solid Phase Extraction / methods*

Substances

  • Fluorobenzenes
  • Herbicides
  • Nitro Compounds
  • 4-chloro-3,5-dinitrobenzotrifluoride
  • Amitrole