Interaction of organotin with piperazine derived self-assembled cylindrical bisdithiocarbamates: spectral and thermal investigations

Spectrochim Acta A Mol Biomol Spectrosc. 2009 Jul;73(1):89-95. doi: 10.1016/j.saa.2009.01.033. Epub 2009 Feb 20.

Abstract

Few organotin complexes of the type R4Sn2L2 where R=CH3 (2), C4H9 (3), C6H5 (4), and Sn2L2Cl4 (5) (L=bis(2,2'-dithiopiperazinato-2,2'-diaminodiethylamine)) have been synthesized and suitably characterized by FT-IR, UV-vis, 1H NMR, 119Sn NMR, ESI-MS, TGA/DSC, microanalysis and room temperature molar conductivity data. On the basis of FT-IR spectral studies, a symmetrical bidentate coordination has been proposed for all the complexes while the absence of any higher peak in the ESI-MS may be corroborated with the formation of binuclear complexes. On the basis of 119Sn NMR spectroscopy, six-coordinate geometry has been observed for the Sn-center in all the complexes. The TGA/DSC profile of the complexes implies their higher stability than its precursor. However, on the basis of IDT values the stability order of the organotin complexes was found to be 4>3>2. The room temperature conductivity values of the 1 mM solution of the ligand and its complexes are found to be comparable with that of non-ionic complexes.

MeSH terms

  • Calorimetry, Differential Scanning
  • Chemical Phenomena
  • Molecular Structure
  • Organotin Compounds / chemistry*
  • Piperazine
  • Piperazines / chemistry*
  • Spectrometry, Mass, Electrospray Ionization
  • Spectrophotometry
  • Temperature*
  • Thiocarbamates / chemistry*

Substances

  • Organotin Compounds
  • Piperazines
  • Thiocarbamates
  • Piperazine